So many to choose from, so many masterpieces: Alien, Poltergeist, The Blue Max, Capricorn One, The Edge, Islands in the stream, The Omen, Planet of the Apes, Freud, Secret of Nimh, Total Recall, Night Crossing ...
But I think my absolutely favourite is Legend. Pure magic. It's a full-blown romantic, big symphonic score with choir and soloist. One of the things I'm always being fascinated of is how masterfully Goldsmith integrated synthesizers into this score. Not as a cheesy or rhythmical accompaniment he does so often, but as equal instruments within the Orchestra, expanding wildely the colours. With this he creates a soundscape worthy of the gorgeous and dreamlike pictures of the film.
So sad (and unforgivable) that Scott replaced the Goldsmith Score with the pure synthesizer score of Tangerine Dream (for the american cut).